Emerging two dimensional metastable-phase oxides: insights and prospects in synthesis and catalysis
Jiaqi Su1, Xiaoqing Huang2*（黄小青）, Qi Shao1*（邵琪）
1Collegeof Chemistry, ChemicalEngineeringand MaterialsScience,SoochowUniversityJiangsu215123(P. R. China)
2StateKey Laboratoryof PhysicalChemistryof SolidSurfaces,Collegeof Chemistryand ChemicalEngineering,XiamenUniversityXiamen361005(P. R. China)
Angew. Chem.Int. Ed.2024,63,e202318028(2 of 15)
Abstract:Since the discovery of graphene, the development of new two-dimensional (2D) materials has received considerable interest. Recently, as a newly emerging member of the 2D family, 2D metastable-phase oxides that combine the unique advantages of metal oxides, 2D structures, and metastable-phase materials have shown enormous potential in various catalytic reactions. In this review, the potential of various 2D materials to form a metastable-phase is predicted. The advantages of 2D metastable-phase oxides for advanced applications, reliable methods of synthesizing 2D metastable-phase oxides, and the application of these oxides in different catalytic reactions are presented. Finally, the challenges associated with 2D metastable-phase oxides and future perspectives are discussed.
链接：https://onlinelibrary.wiley.com/doi/10.1002/anie.202318028
